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I think microtonal stuff is rather interesting, but I haven't really heard any interesting music written with it without it sounding like 12-tone music "detuned" (both nature and nuture has enforced this perception upon us) - probably because it's not really intuitive to extend the theory behind equal temperment 12-tone music to other scales (or rather, a successful and consistent method in writing music regardless of the tuning). The only thing I can think of is serialization, but then again, even 12-tone serial music can be somewhat of a hit-and-miss.
I haven' really had much chance to experiment with microtones, but so far I've only used for "color". I've be really interested in a MIDI sequencer/notator with user-friendly microtonal support, but haven't seen any yet (closest thing to it would be Scala, but it's a rather complex program, and you can't directly sequence with it).
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